Researchers from the University of Oklahoma (OU) and Northwestern University recently addressed light emission problems prevalent in quantum applications. Quantum light sources can flicker like stars and fade out like, but the team's recent research proves that adding a covering to one of these light sources, called a colloidal quantum dot, can cause them to shine without faltering, opening the door to new, affordable quantum possibilities.
Sythensized QDs suspended in solvents under laser irradiation. Image credit: Eurekalert and Jonathan Kyncl
The study, led by OU Assistant Professor Yitong Dong, demonstrates that adding a crystalized molecular layer to QDs made of perovskite neutralizes surface defects and stabilizes the surface lattices. Doing so prevents them from darkening or blinking.
“In quantum computing, you must be able to control how many photons are emitted at any given time,” he said. “QDs are notoriously unstable, so we worked to create a crystal covering that could stabilize their quantum emissions. This material is ideal because it is inexpensive to use and scale and is efficient at room temperature.”
Quantum dots have historically had several problems. First, their surfaces can easily become defective. These defects can cause the QDs to fail, often after only 10-20 minutes of use. The crystal coverings deployed by Dong and his collaborators extend the continuous photon emission of QDs to more than 12 hours without any decay, and virtually no blinking.
Second, single photon emitters have traditionally operated at extremely low cryogenic temperatures. In fact, they typically require liquid helium at -452 degrees Fahrenheit, making them impractical for most real-world applications. This research, however, demonstrates that perovskite QDs achieve nearly 100% efficiency at room temperature. This breakthrough makes them significantly easier, cheaper and more appealing to use.
“Although there has been real interest in the exotic optical properties of this material, the sophistication needed to fabricate a single photon emitter was cost-prohibitive,” Dong said. “But since perovskite QDs can be used at normal temperatures and synthesized for very little cost, we believe they could become the photonic chip light source for future quantum computing and quantum communication devices.”
According to Dong, these findings could pave the way for future quantum emitter designs that extend beyond this specific material or molecular structure.
“In my opinion, our research has profound implications for the quantum field,” he said. “We’ve found a way to stabilize these QDs using organic and inorganic molecular crystals, opening the door for others to explore the fundamental optical properties and fundamental physics of these materials. It’s really exciting.”
